Excited states decay in carbon nanotubes
Vasili Perebeinos
LS 2008
We used the high local electric fields at the junction between the suspended and supported parts of a single carbon nanotube molecule to produce unusually bright infrared emission under unipolar operation. Carriers were accelerated by band-bending at the suspension interface, and they created excitons that radiatively recombined. This excitation mechanism is ∼1000 times more efficient than recombination of independently injected electrons and holes, and it results from weak electron-phonon scattering and strong electron-hole binding caused by one-dimensional confinement. The ensuing high excitation density allows us to observe emission from higher excited states not seen by photoexcitation. The excitation mechanism of these states was analyzed.
Vasili Perebeinos
LS 2008
Marcus Freitag, Jia Chen, et al.
Physical Review Letters
Marcus Freitag, James C. Tsang, et al.
Nano Letters
Fengnian Xia, Vasili Perebeinos, et al.
Nature Nanotechnology